A continuation of the anthology series “Alfred Hitchcock Presents”, hosted by the master of suspense and featuring thrillers and mysteries.

Richard Kimble is falsely convicted of his wife's murder and given the death penalty. En route to death row, Kimble's train derails and crashes, allowing him to escape and begin a cross-country search for the real killer, a "one-armed man". At the same time, Dr. Kimble is hounded by the authorities, most notably dogged by Police Lieutenant Philip Gerard.

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Agents Napoleon Solo and Illya Kuryakin work for a secret intelligence service working under the auspices of the U.N. Their immediate superior is Mr. Waverly. Together they operate out of a secret base beneath the streets of New York City, and accesses through several cover business such as Del Floria's Tailor Shop and the Masque Club. This secret intelligence service is called U.N.C.L.E. United Network Command for Law and Enforcement.

Sam Casey is an agent for INTERSECT, a government think-tank and operations center specializing in secret missions. While on a diving assignment, Sam was affected by the radiation from an underwater explosion. The radiation rendered him invisible, but INTERSECT devised a way to control his invisibility, by fitting him with a computerized watch that kept him visible. He could, however, shut it off, and become invisible again, for short periods of time. If he did this for more than 15 minutes in any 24 hour period he would die. This ability to become invisible made him a very effective agent.

Professor Joe Howe is a Korean War veteran who is hired to teach English at Channing College. The dean Fred Baker is his mentor as Howe is writing a novel about his experiences. They are frequently involved in the student's lives. Channing, a production of Revue Studios, aired during the same time frame as the first season of NBC's somewhat similar offering, Mr. Novak.

Rags-to-riches tale of an Irish immigrant in late 1800s based on the novel by Taylor Caldwell.

A sophisticated, middle-aged grandmother, wed to a New York law professor, falls in love with a down-to-earth Tennessee farmer.

Agent Sam Casey is in a satellite explosion and the radiation turns him invisible. He gets a watch that keeps him visible, and he uses it to switch from visible to invisible. He is assigned to transport a chemical called Tripolydine, which is purported to be the most efficient fuel; when the cover is blown on that and he uncovers and stops the Tripolydine fraud, he must then stop a terrorist from blowing up race cars.

A bomb on board an airliner has an altitude-sensitive trigger. Unless a ransom is paid, it will explode when the plane descends to land.

Two pilots are hired to reclaim a stolen jet from the son of a South American dictator.